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DOI10.1016/j.atmosenv.2020.118087
Summertime O3 and related health risks in the north China plain: A modeling study using two anthropogenic emission inventories
Chen K.; Wang P.; Zhao H.; Wang P.; Gao A.; Myllyvirta L.; Zhang H.
发表日期2021
ISSN1352-2310
卷号246
英文摘要Ground-level ozone (O3), which is formed by photochemical reactions of nitrogen oxides (NOx) and volatile organic compounds (VOCs), exert adverse effects on human health. In China, the mechanism and influencing factors of high O3 levels are not well understood in China despite the frequent occurrence of extreme episodes in recent years with decreasing concentrations of particulate matter. In this study, the O3 concentrations in summer 2017 in the North China Plain (NCP) are simulated using the Community Multiscale Air Quality (CMAQ) model with anthropogenic emissions from the Multi-resolution Emission Inventory for China (MEIC) and improved Emission Database for Global Atmospheric Research (EDGAR+). Moreover, the performances of the model with the two emission inventories are validated and compared. The simulation using EDGAR+ is found to be highly accurate in predicting O3 in the NCP, whereas that using MEIC has better performance in matching peak concentrations in extreme episodes. Weather conditions, such as high temperature, low relative humidity, and stable conditions, are associated with high O3 concentrations in both inventories. Compared with MEIC, lower NOx emissions (by 200 tons/grid/month) from EDGAR+ induce higher O3 concentrations when VOCs emissions are barely changed (by less than 5 tons/grid/month). In the EDGAR+ scenario, a total of 42,000 and 69,000 premature mortalities are estimated to be caused by O3-related respiratory and cardiovascular diseases, respectively. These values are slightly lower than those in the MEIC scenario, i.e., 50,000 and 80,000, respectively. Megacities, such as Beijing and Tianjin, are classified as high-risk areas, with more than 15,000 mortalities. © 2020 Elsevier Ltd
英文关键词Air quality; Atmospheric humidity; Nitrogen oxides; Photochemical reactions; Volatile organic compounds; Anthropogenic emissions; Atmospheric research; Cardio-vascular disease; Community multi-scale air qualities; Emission inventories; Low relative humidities; Peak concentrations; Premature mortality; Health risks
语种英语
来源期刊Atmospheric Environment
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/169094
作者单位Department of Environmental Science and Engineering, Fudan University, Shanghai, 200438, China; Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Nanjing University of Information Science & Technology, Nanjing, 210044, China; Department of Civil and Environmental Engineering, Louisiana State University, Baton Rouge, LA 70803, United States; Department of Civil and Environmental Engineering, Hong Kong Polytechnic University99907, China; School of Water Resources and Environment, Hebei GEO University, Shijiazhuang, 050031, China; Centre for Research on Energy and Clean Air (CREA), Helsinki, Finland
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Chen K.,Wang P.,Zhao H.,et al. Summertime O3 and related health risks in the north China plain: A modeling study using two anthropogenic emission inventories[J],2021,246.
APA Chen K..,Wang P..,Zhao H..,Wang P..,Gao A..,...&Zhang H..(2021).Summertime O3 and related health risks in the north China plain: A modeling study using two anthropogenic emission inventories.Atmospheric Environment,246.
MLA Chen K.,et al."Summertime O3 and related health risks in the north China plain: A modeling study using two anthropogenic emission inventories".Atmospheric Environment 246(2021).
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