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DOI10.5194/acp-20-15285-2020
Weaker cooling by aerosols due to dust-pollution interactions
Klingmüller K.; Karydis V.A.; Bacer S.; Stenchikov G.L.; Lelieveld J.
发表日期2020
ISSN1680-7316
起始页码15285
结束页码15295
卷号20期号:23
英文摘要The interactions between aeolian dust and anthropogenic air pollution, notably chemical ageing of mineral dust and coagulation of dust and pollution particles, modify the atmospheric aerosol composition and burden. Since the aerosol particles can act as cloud condensation nuclei, this affects the radiative transfer not only directly via aerosol-radiation interactions, but also indirectly through cloud adjustments. We study both radiative effects using the global ECHAM/MESSy atmospheric chemistry-climate model (EMAC) which combines the Modular Earth Submodel System (MESSy) with the European Centre/Hamburg (ECHAM) climate model. Our simulations show that dust- pollution-cloud interactions reduce the condensed water path and hence the reflection of solar radiation. The associated climate warming outweighs the cooling that the dust-pollution interactions exert through the direct radiative effect. In total, this results in a net warming by dust-pollution interactions which moderates the negative global anthropogenic aerosol forcing at the top of the atmosphere by (0.2-0.1) Wm-2. © 2020 BMJ Publishing Group. All rights reserved.
英文关键词aerosol; aerosol composition; air quality; atmospheric pollution; climate modeling; coagulation; computer simulation; cooling; dust; numerical model; radiative transfer
语种英语
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/168898
作者单位Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, 55128, Germany; Forschungszentrum Jülich GmbH, IEK-8, Jülich, 52425, Germany; LEGI, Université Grenoble Alpes, CNRS, Grenoble INP, Grenoble, France; King Abdullah University of Science and Technology, Thuwal, 23955-6900, Saudi Arabia; Cyprus Institute, P.O. Box 27456, Nicosia, 1645, Cyprus
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Klingmüller K.,Karydis V.A.,Bacer S.,et al. Weaker cooling by aerosols due to dust-pollution interactions[J],2020,20(23).
APA Klingmüller K.,Karydis V.A.,Bacer S.,Stenchikov G.L.,&Lelieveld J..(2020).Weaker cooling by aerosols due to dust-pollution interactions.Atmospheric Chemistry and Physics,20(23).
MLA Klingmüller K.,et al."Weaker cooling by aerosols due to dust-pollution interactions".Atmospheric Chemistry and Physics 20.23(2020).
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