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DOI | 10.1038/s41893-019-0446-4 |
Surface-engineered sponges for recovery of crude oil microdroplets from wastewater | |
Cherukupally P.; Sun W.; Wong A.P.Y.; Williams D.R.; Ozin G.A.; Bilton A.M.; Park C.B. | |
发表日期 | 2020 |
ISSN | 2398-9629 |
起始页码 | 136 |
结束页码 | 143 |
卷号 | 3期号:2 |
英文摘要 | In the United States, the oil industry produces over 15 billion barrels of wastewater contaminated with crude oil microdroplets annually. Current methods are ineffective for the removal of these microdroplets at the variable pH conditions commonly found in wastewater. Here, an innovative surface-engineered sponge (SEnS) that synergistically combines surface chemistry, charge and roughness, provides a solution to this problem. Over broad pH conditions, the SEnS rapidly adsorbed oil microdroplets with 95–99% removal efficiency, predominantly facilitated by Lifshitz–van der Waals forces. At the optimum pH, 92% of the oil was adsorbed within 10 min. The oil was subsequently recovered by solvent extraction under ambient conditions, and the cleaned SEnS was reused for oil microdroplets adsorption ten times. The combined efficacy and reusability can enable large-scale removal and recovery of crude oil microdroplets from wastewater. © 2019, The Author(s), under exclusive licence to Springer Nature Limited. |
语种 | 英语 |
scopus关键词 | pH; Recovery; Reusability; Solvent extraction; Surface chemistry; Van der Waals forces; Ambient conditions; Micro droplets; Oil industries; Optimum pH; pH condition; Removal and recoveries; Removal efficiencies; Crude oil |
来源期刊 | Nature Sustainability |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/163119 |
作者单位 | Department of Mechanical and Industrial Engineering, University of Toronto, Toronto, ON, Canada; Department of Chemical Engineering, Imperial College London, London, United Kingdom; Department of Chemistry, University of Toronto, Toronto, ON, Canada; State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University, Hangzhou, China |
推荐引用方式 GB/T 7714 | Cherukupally P.,Sun W.,Wong A.P.Y.,et al. Surface-engineered sponges for recovery of crude oil microdroplets from wastewater[J],2020,3(2). |
APA | Cherukupally P..,Sun W..,Wong A.P.Y..,Williams D.R..,Ozin G.A..,...&Park C.B..(2020).Surface-engineered sponges for recovery of crude oil microdroplets from wastewater.Nature Sustainability,3(2). |
MLA | Cherukupally P.,et al."Surface-engineered sponges for recovery of crude oil microdroplets from wastewater".Nature Sustainability 3.2(2020). |
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