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DOI | 10.1039/d0ee01790f |
Quantitative isotope measurements in heterogeneous photocatalysis and electrocatalysis | |
Lin Y.; Deng C.; Wu L.; Zhang Y.; Chen C.; Ma W.; Zhao J. | |
发表日期 | 2020 |
ISSN | 1754-5692 |
起始页码 | 2602 |
结束页码 | 2617 |
卷号 | 13期号:9 |
英文摘要 | Heterogeneous photocatalysis and electrocatalysis have attracted tremendous interest in energy chemistry including CO2 reduction, N2 fixation, water oxidation, oxygen reduction, organic transformations, etc. The molecular-level understanding of reaction mechanisms in photocatalysis and electrocatalysis is pivotal to facilitate these processes, and the quantitative isotope measurement provides such a toolbox. Herein, we summarize the theory of two kinds of important isotope measurements (i.e., kinetic isotope effect and isotope labeling methods) and then review their important applications in photocatalytic/electrocatalytic CO2 reduction, N2 fixation, water oxidation, oxygen reduction and organic transformations on heterogeneous catalysts. Future prospects for quantitative isotope measurements are also presented. This journal is © The Royal Society of Chemistry. |
语种 | 英语 |
scopus关键词 | Carbon dioxide; Electrocatalysis; Electrolytic reduction; Molecular oxygen; Photocatalysis; Rate constants; Energy chemistry; Future prospects; Heterogeneous catalyst; Heterogeneous photocatalysis; Isotope measurements; Kinetic isotope effects; Organic transformations; Reaction mechanism; Isotopes; catalysis; catalyst; electrochemistry; heterogeneity; isotopic analysis; measurement method; photochemistry; quantitative analysis |
来源期刊 | Energy and Environmental Science |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/162636 |
作者单位 | Key Laboratory of Photochemistry, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China; University of Chinese Academy of Sciences, Beijing, 100049, China |
推荐引用方式 GB/T 7714 | Lin Y.,Deng C.,Wu L.,et al. Quantitative isotope measurements in heterogeneous photocatalysis and electrocatalysis[J],2020,13(9). |
APA | Lin Y..,Deng C..,Wu L..,Zhang Y..,Chen C..,...&Zhao J..(2020).Quantitative isotope measurements in heterogeneous photocatalysis and electrocatalysis.Energy and Environmental Science,13(9). |
MLA | Lin Y.,et al."Quantitative isotope measurements in heterogeneous photocatalysis and electrocatalysis".Energy and Environmental Science 13.9(2020). |
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