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DOI10.1073/pnas.1719443115
Multidimensional photon correlation spectroscopy of cavity polaritons
Dorfman K.E.; Mukamel S.
发表日期2018
ISSN0027-8424
起始页码1451
结束页码1456
卷号115期号:7
英文摘要The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes–Cummings model. © 2018 National Academy of Sciences. All Rights Reserved.
英文关键词Cavity polaritons; Multidimensional spectroscopy; Photon correlation
语种英语
scopus关键词analytic method; Article; cavity polariton; controlled study; gated single photon emission computed tomography; oscillation; photobiology; photochemistry; photon correlation spectroscopy; physical phenomena; prediction; priority journal; scanning tunneling microscopy; single photon emission computed tomography; article; cross coupling reaction; energy transfer; optical spectroscopy; radiation field
来源期刊Proceedings of the National Academy of Sciences of the United States of America
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/160545
作者单位Dorfman, K.E., State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai, 200062, China; Mukamel, S., Department of Chemistry, University of California, Irvine, CA 92697, United States, Department of Physics and Astronomy, University of California, Irvine, CA 92697, United States
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Dorfman K.E.,Mukamel S.. Multidimensional photon correlation spectroscopy of cavity polaritons[J],2018,115(7).
APA Dorfman K.E.,&Mukamel S..(2018).Multidimensional photon correlation spectroscopy of cavity polaritons.Proceedings of the National Academy of Sciences of the United States of America,115(7).
MLA Dorfman K.E.,et al."Multidimensional photon correlation spectroscopy of cavity polaritons".Proceedings of the National Academy of Sciences of the United States of America 115.7(2018).
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