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DOI | 10.1073/pnas.1719443115 |
Multidimensional photon correlation spectroscopy of cavity polaritons | |
Dorfman K.E.; Mukamel S. | |
发表日期 | 2018 |
ISSN | 0027-8424 |
起始页码 | 1451 |
结束页码 | 1456 |
卷号 | 115期号:7 |
英文摘要 | The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes–Cummings model. © 2018 National Academy of Sciences. All Rights Reserved. |
英文关键词 | Cavity polaritons; Multidimensional spectroscopy; Photon correlation |
语种 | 英语 |
scopus关键词 | analytic method; Article; cavity polariton; controlled study; gated single photon emission computed tomography; oscillation; photobiology; photochemistry; photon correlation spectroscopy; physical phenomena; prediction; priority journal; scanning tunneling microscopy; single photon emission computed tomography; article; cross coupling reaction; energy transfer; optical spectroscopy; radiation field |
来源期刊 | Proceedings of the National Academy of Sciences of the United States of America |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/160545 |
作者单位 | Dorfman, K.E., State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai, 200062, China; Mukamel, S., Department of Chemistry, University of California, Irvine, CA 92697, United States, Department of Physics and Astronomy, University of California, Irvine, CA 92697, United States |
推荐引用方式 GB/T 7714 | Dorfman K.E.,Mukamel S.. Multidimensional photon correlation spectroscopy of cavity polaritons[J],2018,115(7). |
APA | Dorfman K.E.,&Mukamel S..(2018).Multidimensional photon correlation spectroscopy of cavity polaritons.Proceedings of the National Academy of Sciences of the United States of America,115(7). |
MLA | Dorfman K.E.,et al."Multidimensional photon correlation spectroscopy of cavity polaritons".Proceedings of the National Academy of Sciences of the United States of America 115.7(2018). |
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