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DOI10.1073/pnas.1811873115
Itinerant ferromagnetism of the Pd-terminated polar surface of PdCoO 2
Mazzola F.; Sunko V.; Khim S.; Rosner H.; Kushwaha P.; Clark O.J.; Bawden L.; Marković I.; Kim T.K.; Hoesch M.; Mackenzie A.P.; King P.D.C.
发表日期2018
ISSN0027-8424
起始页码12956
结束页码12960
卷号115期号:51
英文摘要The ability to modulate the collective properties of correlated electron systems at their interfaces and surfaces underpins the burgeoning field of “designer” quantum materials. Here, we show how an electronic reconstruction driven by surface polarity mediates a Stoner-like magnetic instability to itinerant ferromagnetism at the Pd-terminated surface of the nonmagnetic delafossite oxide metal PdCoO 2 . Combining angle-resolved photoemission spectroscopy and density-functional theory calculations, we show how this leads to a rich multiband surface electronic structure. We find similar surface state dispersions in PdCrO 2 , suggesting surface ferromagnetism persists in this sister compound despite its bulk antiferromagnetic order. © 2018 National Academy of Sciences. All rights reserved.
英文关键词Angle-resolved photoemission; Delafossite; Electronic reconstruction; Itinerant ferromagnetism; Transition-metal oxide
语种英语
scopus关键词cobalt; copper oxide; iron oxide; palladium; angle resolved photoemission spectroscopy; Article; crystal structure; magnetism; photoelectron spectroscopy; priority journal; surface property; theoretical study; X ray photoemission spectroscopy
来源期刊Proceedings of the National Academy of Sciences of the United States of America
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/160436
作者单位Mazzola, F., Scottish Universities Physics Alliance, School of Physics and Astronomy, University of St. Andrews, St. Andrews, KY16 9SS, United Kingdom; Sunko, V., Scottish Universities Physics Alliance, School of Physics and Astronomy, University of St. Andrews, St. Andrews, KY16 9SS, United Kingdom, Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany; Khim, S., Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany; Rosner, H., Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany; Kushwaha, P., Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany; Clark, O.J., Scottish Universities Physics Alliance, School of Physics and Astronomy, University of St. Andrews, St. Andrews, KY16 9SS, United Kingdom; Bawden, L., Scottish Universities Physics Alliance, School of Physics and Astronomy, University of St. Andrews, St. Andrews, KY16 9SS, United Kingdom; Marković, I., Scottish Universities Physics Alliance, School of Physics...
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GB/T 7714
Mazzola F.,Sunko V.,Khim S.,et al. Itinerant ferromagnetism of the Pd-terminated polar surface of PdCoO 2[J],2018,115(51).
APA Mazzola F..,Sunko V..,Khim S..,Rosner H..,Kushwaha P..,...&King P.D.C..(2018).Itinerant ferromagnetism of the Pd-terminated polar surface of PdCoO 2.Proceedings of the National Academy of Sciences of the United States of America,115(51).
MLA Mazzola F.,et al."Itinerant ferromagnetism of the Pd-terminated polar surface of PdCoO 2".Proceedings of the National Academy of Sciences of the United States of America 115.51(2018).
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