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DOI10.1016/j.apgeochem.2020.104627
Diffusion of polycyclic aromatic hydrocarbons between water and sediment and their ecological risks in Wuhu city, Yangtze River Delta urban agglomerations, China
Xu H.; Wang Q.; Wang X.; Feng W.; Zhu F.
发表日期2020
ISSN2697491
卷号119
英文摘要To understand how black carbon (BC) might affect the nature of polycyclic aromatic hydrocarbons (PAHs) diffusion at the water–sediment interface and how their diffusion process and ecological risks vary in different functional areas due to strong heterogeneity of urban system. 24 pairs of samples (water and sediment) were collected across the watery landscape of Wuhu, China in four functional areas. The results suggested that PAHs concentrations ranged between 6.95 and 43.2 ng/L, with a mean value of 19.8 ng/L in water, and were from 32.8 to 3790 ng/g averaging 690 ng/g in sediment. The primary sources of the PAHs might be coal combustion and biomass combustion as was revealed by Positive Matrix Factorization model. BC can absorb PAHs, especially high-molecular-weight (HMW) PAHs with strong lipophilic properties, into sediment and affect their diffusion trend at water-sediment interface in different functional areas. The coexistence of BC and PAHs will affect the associated risks in aquatic environments. The water has a higher risk in the education and residential area, which was polluted by low-molecular-weight (LMW) PAHs. The sediment risk was mainly manifested in industrial areas, which are contaminated by HMW PAHs that was caused by the presence of BC. These results indicate that it is very significant for ecological risk assessment to understand the pollution status of PAHs in different functional areas and their relationship with BC. © 2020 Elsevier Ltd
英文关键词Aquatic landscape; BC; Diffusion; Ecological risk; PAHs; Water–sediment interface
语种英语
scopus关键词Applied Geochemistry
来源机构中国科学院青藏高原研究所
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/158416
作者单位School of Geography and Tourism, Anhui Normal University, Wuhu, 241003, China; Key Laboratory of Earth Surface Processes and Regional Response in the Yangtze-Huaihe River Basin, Wuhu, 241003, China; Key Laboratory of Tibetan Environment Changes and Land Surface Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China; CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China; University of Chinese Academy of Sciences, China School of Science, Beijing, 100049, China
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Xu H.,Wang Q.,Wang X.,et al. Diffusion of polycyclic aromatic hydrocarbons between water and sediment and their ecological risks in Wuhu city, Yangtze River Delta urban agglomerations, China[J]. 中国科学院青藏高原研究所,2020,119.
APA Xu H.,Wang Q.,Wang X.,Feng W.,&Zhu F..(2020).Diffusion of polycyclic aromatic hydrocarbons between water and sediment and their ecological risks in Wuhu city, Yangtze River Delta urban agglomerations, China.,119.
MLA Xu H.,et al."Diffusion of polycyclic aromatic hydrocarbons between water and sediment and their ecological risks in Wuhu city, Yangtze River Delta urban agglomerations, China".119(2020).
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