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DOI10.1088/1748-9326/ab83aa
Local formation of sulfates contributes to the urban haze with regional transport origin
Lim Y.B.; Seo J.; Kim J.Y.; Kim Y.P.; Jin H.C.
发表日期2020
ISSN17489318
卷号15期号:8
英文摘要Urban particle pollution is affected by not only the emissions of pollutants and secondary aerosol formation through atmospheric chemistry on a local scale, but also the regional transport of particles and precursor gases from highly polluted upwind areas. However, this regional impact on urban particle formation is not well understood. Wintertime haze events occur at Seoul, Korea through the combination of regional transport from China and local formation at Seoul. We perform thermodynamic model simulations based on inorganic component measurements of haze particles collected at Seoul and Deokjeok Island (upwind background). Results suggest that in the downwind area (Seoul) the local formation of sulfates increases the mass concentrations of transported particles through the gas-particle partitioning of semivolatile nitric acid (HNO3) and ammonia (NH3). Therefore, this synergetic effect of the local sulfate formation on urban haze with regional transport must be considered in implementing effective particle reduction controls for urban sustainability. © 2020 The Author(s). Published by IOP Publishing Ltd.
英文关键词East Asian haze; gas particle partitioning of semivolatile inorganic species; regional transport
语种英语
scopus关键词Ammonia; Atmospheric chemistry; Atmospheric movements; Nitric acid; Pollution; Sulfur compounds; Gas-particle partitioning; Inorganic components; Mass concentration; Particle reduction; Regional transport; Secondary aerosols; Thermodynamic model; Urban sustainability; Urban transportation; aerosol formation; atmospheric chemistry; atmospheric pollution; concentration (composition); haze; sulfate; urban pollution; China; Deokjeok Island; Incheon [South Korea]; Seoul; South Korea
来源期刊Environmental Research Letters
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/153910
作者单位Department of Chemical Engineering and Material Science, Ewha Womans University, Seoul, 03760, South Korea; Environment, Health and Welfare Research Center, Korea Institute of Science and Technology, Seoul, 02792, South Korea; School of Earth and Environmental Sciences, Seoul National University, Seoul, 08826, South Korea
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Lim Y.B.,Seo J.,Kim J.Y.,et al. Local formation of sulfates contributes to the urban haze with regional transport origin[J],2020,15(8).
APA Lim Y.B.,Seo J.,Kim J.Y.,Kim Y.P.,&Jin H.C..(2020).Local formation of sulfates contributes to the urban haze with regional transport origin.Environmental Research Letters,15(8).
MLA Lim Y.B.,et al."Local formation of sulfates contributes to the urban haze with regional transport origin".Environmental Research Letters 15.8(2020).
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