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DOI10.5194/acp-20-13425-2020
Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018
Lee H.; Lee K.; Rene Lunder C.; Krejci R.; Aas W.; Park J.; Park K.-T.; Yong Lee B.; Yoon Y.J.; Park K.
发表日期2020
ISSN16807316
起始页码13425
结束页码13441
卷号20期号:21
英文摘要We conducted continuous measurements of nanoparticles down to 3 nm size in the Arctic at Mount Zeppelin, Ny Ålesund, Svalbard, from October 2016 to December 2018, providing a size distribution of nanoparticles (3-60 nm). A significant number of nanoparticles as small as 3 nm were often observed during new particle formation (NPF), particularly in summer, suggesting that these were likely produced near the site rather than being transported from other regions after growth. The average NPF frequency per year was 23 %, having the highest percentage in August (63 %). The average formation rate (J ) and growth rate (GR) for 3-7 nm particles were 0.04 cm-3 s-1 and 2.07 nm h-1, respectively. Although NPF frequency in the Arctic was comparable to that in continental areas, the J and GR were much lower. The number of nanoparticles increased more frequently when air mass originated over the south and southwest ocean regions; this pattern overlapped with regions having strong chlorophyll a concentration and dimethyl sulfide (DMS) production capacity (southwest ocean) and was also associated with increased NH3 and H2SO4 concentration, suggesting that marine biogenic sources were responsible for gaseous precursors to NPF. Our results show that previously developed NPF occurrence criteria (low loss rate and high cluster growth rate favor NPF) are also applicable to NPF in the Arctic. © Author(s) 2020.
语种英语
scopus关键词aerosol formation; biogenic emission; measurement method; nanoparticle; particle size; size distribution; Arctic; Arctic Ocean; Ny-Alesund; Spitsbergen; Svalbard; Svalbard and Jan Mayen
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/152833
作者单位School of Earth Sciences and Environmental Engineering, Gwangju Institute of Science and Technology, 123 Cheomdangwagiro, Buk-gu, Gwangju, 61005, South Korea; Department for Atmospheric and Climate Research, NILU-Norwegian Institute for Air Research, Kjeller, Norway; Department of Environmental Sciences and the Bolin Centre for Climate Research, Stockholm University, Stockholm, 106 91, Sweden; Korea Polar Research Institute, 26, Songdo Mirae-ro, Yeonsu-Gu, Incheon, South Korea
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Lee H.,Lee K.,Rene Lunder C.,et al. Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018[J],2020,20(21).
APA Lee H..,Lee K..,Rene Lunder C..,Krejci R..,Aas W..,...&Park K..(2020).Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018.Atmospheric Chemistry and Physics,20(21).
MLA Lee H.,et al."Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018".Atmospheric Chemistry and Physics 20.21(2020).
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