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DOI10.1016/j.quascirev.2019.106076
A 10;000-year record of trace metal and metalloid (Cu; Hg; Sb; Pb) deposition in a western Alpine lake (Lake Robert; France): Deciphering local and regional mining contamination
Elbaz-Poulichet F.; Guédron S.; Anne-Lise D.; Freydier R.; Perrot V.; Rossi M.; Piot C.; Delpoux S.; Sabatier P.
发表日期2020
ISSN0277-3791
卷号228
英文摘要Concentrations of trace metals and metalloids (Cu, Hg, Sb, Pb), major elements, stable Pb and C isotope ratios, total organic carbon (TOC), C/N atomic ratios, were analyzed in two sediment cores encompassing 10,000 years of sedimentation sampled in Lake Robert (French Alps). The results showed that the establishment of a soil cover and vegetation during the Holocene climatic optimum increased Cu and Hg deposition in sediments. Results also enabled reconstruction of the history and local vs regional origins of pollution. During the Bronze Age (1800–1000 BC), Cu mining activities increased Hg and Sb accumulation rates (AR) by a factor of 7 (Hg) and 9 (Sb) compared to pre-Bronze Age values. The rise in Hg AR was equivalent to that of the industrial era highlighting a major local Hg point source not recorded in regional archives. During the Iron Age, Pb pollution was attributed to Sicilian ores whereas during the Roman Empire Pb pollution had the isotopic signature of Spanish Pb ores. During the Medieval period (ca. AD 1200), Pb and Hg pollution was due to the exploitation of the local Ag–Pb mines. Finally, during the industrial era, metal accumulations rates were 90 (Pb), 5 (Hg) and 20 (Sb) times higher than those in the pre-Bronze Age. The isotopic composition of Pb reflected mixed sources including industrial Pb and gasoline Pb. Synchronously, the increase in Sb and Hg pollution is attributed to global and regional atmospheric pollution. © 2019 Elsevier Ltd
英文关键词Alpine lake; Antimony; Bronze age pollution; Copper; Holocene sediment record; Lead isotopes; Mercury
语种英语
scopus关键词Antimony; Bronze; Copper; Deposition; Isotopes; Lakes; Mercury (metal); Metals; Organic carbon; Sediments; Soils; Trace elements; Alpine lakes; Atmospheric pollution; Bronze age; Holocene sediments; Isotopic composition; Isotopic signatures; Lead isotope; Total Organic Carbon; Lake pollution; antimony; Bronze Age; copper; glacial sedimentation; isotopic composition; lead isotope; mercury (element); organic carbon; sedimentation; total organic carbon; trace metal; Alps; France
来源期刊Quaternary Science Reviews
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/151639
作者单位Hydrosciences, Univ. Montpellier, CNRS, IRD, Montpellier, France; Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, IRD, IFSTTAR, ISTerre, Grenoble, 38000, France; Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, EDYTEM, Chambéry, 73000, France; LCME, Univ. Savoie Mont-Blanc, Le Bourget du Lac, 73376, France
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Elbaz-Poulichet F.,Guédron S.,Anne-Lise D.,et al. A 10;000-year record of trace metal and metalloid (Cu; Hg; Sb; Pb) deposition in a western Alpine lake (Lake Robert; France): Deciphering local and regional mining contamination[J],2020,228.
APA Elbaz-Poulichet F..,Guédron S..,Anne-Lise D..,Freydier R..,Perrot V..,...&Sabatier P..(2020).A 10;000-year record of trace metal and metalloid (Cu; Hg; Sb; Pb) deposition in a western Alpine lake (Lake Robert; France): Deciphering local and regional mining contamination.Quaternary Science Reviews,228.
MLA Elbaz-Poulichet F.,et al."A 10;000-year record of trace metal and metalloid (Cu; Hg; Sb; Pb) deposition in a western Alpine lake (Lake Robert; France): Deciphering local and regional mining contamination".Quaternary Science Reviews 228(2020).
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