气候变化领域集成服务门户(CCPortal): Mercury anomalies across the Palaeocene-Eocene Thermal Maximum

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DOI	10.5194/cp-15-217-2019
	Mercury anomalies across the Palaeocene-Eocene Thermal Maximum
	Jones M.T.; Percival L.M.E.; Stokke E.W.; Frieling J.; Mather T.A.; Riber L.; Schubert B.A.; Schultz B.; Tegner C.; Planke S.; Svensen H.H.
发表日期	2019
ISSN	18149324
起始页码	217
结束页码	236
卷号	15 期号:1
英文摘要	Large-scale magmatic events like the emplacement of the North Atlantic Igneous Province (NAIP) are often coincident with periods of extreme climate change such as the Palaeocene-Eocene Thermal Maximum (PETM). One proxy for volcanism in the geological record that is receiving increased attention is the use of mercury (Hg) anomalies. Volcanic eruptions are among the dominant natural sources of Hg to the environment; thus, elevated Hg=TOC values in the sedimentary rock record may reflect an increase in volcanic activity at the time of deposition. Here we focus on five continental shelf sections located around the NAIP in the Palaeogene. We measured Hg concentrations, total organic carbon (TOC) contents, and δ13C values to assess how Hg deposition fluctuated across the PETM carbon isotope excursion (CIE). We find a huge variation in Hg anomalies between sites. The Grane field in the North Sea, the most proximal locality to the NAIP analysed, shows Hg concentrations up to 90 100 ppb (Hg=TOC D 95 700 ppb wt %-1) in the early Eocene. Significant Hg=TOC anomalies are also present in Danish (up to 324 ppb wt %-1) and Svalbard (up to 257 ppb wt %-1) sections prior to the onset of the PETM and during the recovery period, while the Svalbard section also shows a continuous Hg=TOC anomaly during the body of the CIE. The combination with other tracers of volcanism, such as tephra layers and unradiogenic Os isotopes, at these localities suggests that the Hg=TOC anomalies reflect pulses of magmatic activity. In contrast, we do not observe clear Hg anomalies on the New Jersey shelf (Bass River) or the Arctic Ocean (Lomonosov Ridge). This large spatial variance could be due to more regional Hg deposition. One possibility is that phreatomagmatic eruptions and hydrothermal vent complexes formed during the emplacement of sills led to submarine Hg release, which is observed to result in limited distribution in the modern era. The Hg=TOC anomalies in strata deposited prior to the CIE may suggest that magmatism linked to the emplacement of the NAIP contributed to the initiation of the PETM. However, evidence for considerable volcanism in the form of numerous tephra layers and Hg=TOC anomalies post-PETM indicates a complicated relationship between LIP volcanism and climate. Factors such as climate system feedbacks, changes to the NAIP emplacement style, and/or varying magma production rates may be key to both the onset and cessation of hyperthermal conditions during the PETM. However, processes such as diagen esis and organic matter sourcing can have a marked impact on Hg=TOC ratios and need to be better constrained before the relationship between Hg anomalies and volcanic activity can be considered irrefutable. © 2019 Author(s).
语种	英语
scopus关键词	anomaly; climate change; continental shelf; deposition; diagenesis; emplacement; extreme event; geological record; Hypsithermal; igneous province; mercury (element); Paleocene-Eocene boundary; proxy climate record; sedimentary rock; spatial variation; tephra; underwater environment; volcanic eruption; volcanism; Arctic Ocean; Atlantic Ocean; Bass River; Lomonosov Ridge; New Jersey; New Jersey Shelf; United States
来源期刊	Climate of the Past
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/146857
作者单位	Centre for Earth Evolution and Dynamics (CEED), University of Oslo, P.O. Box 1028 Blindern, Oslo, 0315, Norway; Department of Earth Sciences, University of Oxford, South Parks Road, Oxford, OX1 3AN, United Kingdom; Department of Earth Sciences, Utrecht University, Princetonlaan 8a, Utrecht, 3584 CB, Netherlands; Department of Geosciences, University of Oslo, P.O. Box 1047 Blindern, Oslo, 0316, Norway; School of Geosciences, University of Louisiana at Lafayette, Hamilton Hall #323, 611 McKinley St., Lafayette, LA 70504, United States; Museum Salling-Fur Museum, Fur, 7884, Denmark; Department of Geoscience, Aarhus University, Building 1672, Høegh-Guldbergs Gade 2, Aarhus, 8000, Denmark; Volcanic Basin Petroleum Research (VBPR AS), Forskningsparken, Gaustadalléen 21, Oslo, 0349, Norway; Vrije Universitet Brussel, Pleinlaan 2, Brussels, 1050, Belgium
推荐引用方式 GB/T 7714	Jones M.T.,Percival L.M.E.,Stokke E.W.,et al. Mercury anomalies across the Palaeocene-Eocene Thermal Maximum[J],2019,15(1).
APA	Jones M.T..,Percival L.M.E..,Stokke E.W..,Frieling J..,Mather T.A..,...&Svensen H.H..(2019).Mercury anomalies across the Palaeocene-Eocene Thermal Maximum.Climate of the Past,15(1).
MLA	Jones M.T.,et al."Mercury anomalies across the Palaeocene-Eocene Thermal Maximum".Climate of the Past 15.1(2019).