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DOI10.1016/j.atmosres.2020.105344
Source apportionment of volatile organic compounds: Implications to reactivity; ozone formation; and secondary organic aerosol potential
Zheng H.; Kong S.; Chen N.; Niu Z.; Zhang Y.; Jiang S.; Yan Y.; Qi S.
发表日期2021
ISSN0169-8095
卷号249
英文摘要Volatile organic compounds (VOCs) are important contributors to atmospheric chemical reactivity rate (LOH), ozone formation potential (OFP), and secondary organic aerosol formation potential (SOAP). The purpose of this study was to determine the contributions of different VOC sources to LOH, OFP, and SOAP using positive matrix factorization (PMF) model. Hourly observation of ambient VOCs at a megacity of Central China was conducted for one month in winter. The LOH, OFP, and SOAP of VOC species were firstly estimated. The PMF model was then used to apportion their sources. Five VOC sources including solvent usage, gasoline evaporation, combustion sources, vehicle emissions, and industrial sources were apportioned with their average contributions of 11.6%, 14.2%, 39.0%, 22.5%, and 12.6%, respectively. Industrial sources were the highest contributors to the LOH and SOAP with average contributions of 32.2% and 32.8%, respectively, while vehicle emissions contributed most to the OFP (27.8%). This study highlighted that the VOCs and ozone pollution control should give priority to the reactivity (OFP and SOAP) based strategies rather than concentration contribution-based strategies. © 2020 Elsevier B.V.
英文关键词Ozone formation potential; Positive matrix factorization; Secondary organic aerosol; Volatile organic compounds
语种英语
scopus关键词Aerosols; Factorization; Industrial emissions; Ozone; Pollution control; Volatile organic compounds; Combustion sources; Industrial sources; Ozone formation; Ozone formation potentials; Positive matrix factorization models; Secondary organic aerosols; Source apportionment; Vehicle emission; Organic solvents
来源期刊Atmospheric Research
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/145210
作者单位Department of Atmospheric Sciences, School of Environmental Studies, China University of Geosciences, Wuhan, 430078, China; Department of Environmental Science and Engineering, School of Environmental Studies, China University of Geosciences, Wuhan, 430078, China; Eco-Environmental Monitoring Centre of Hubei Province, Wuhan, 430072, China; Research Centre for Complex Air Pollution of Hubei Province, Wuhan, 430078, China
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Zheng H.,Kong S.,Chen N.,et al. Source apportionment of volatile organic compounds: Implications to reactivity; ozone formation; and secondary organic aerosol potential[J],2021,249.
APA Zheng H..,Kong S..,Chen N..,Niu Z..,Zhang Y..,...&Qi S..(2021).Source apportionment of volatile organic compounds: Implications to reactivity; ozone formation; and secondary organic aerosol potential.Atmospheric Research,249.
MLA Zheng H.,et al."Source apportionment of volatile organic compounds: Implications to reactivity; ozone formation; and secondary organic aerosol potential".Atmospheric Research 249(2021).
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