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DOI10.1016/j.atmosenv.2020.117896
Revealing the origin of fine particulate matter in the Sichuan Basin from a source-oriented modeling perspective
Qiao X.; Yuan Y.; Tang Y.; Ying Q.; Guo H.; Zhang Y.; Zhang H.
发表日期2021
ISSN13522310
卷号244
英文摘要The Sichuan Basin (SCB) with 18 cities is one of the regions that are greatly affected by PM2.5 (i.e., particulate matter (PM) with an aerodynamic equivalent diameter less than or equal to 2.5 μm) in China. In this study, we used the Weather Research Forecasting (WRF) model and a source-oriented version of the Community Multiscale Air Quality (CMAQ) model to quantify the contributions from different sectors and regions to PM2.5 for the SCB in 2015. The annual PM2.5 concentrations in the 18 SCB urban centers (i.e., the central urban areas) are 42–112 μg m−3, much higher than the World Health Organization (WHO) guideline (10 μg m−3) and having 20–86, 6–17, and 6–10 μg m−3 due to SCB, non-SCB, and unidentified emissions, respectively. Non-SCB emissions can contribute up to 87 μg m−3 to 24-h PM2.5 concentrations for an urban center. Industrial and residential activities are the largest sectors for annual PM2.5 concentrations in the urban centers, and each of them contributes ~25%–50%. The combined residential and industrial contributions (>~60%) are always much higher than that from each of the other sources on PM2.5 pollution and extreme pollution days (>75 and > 150 μg m−3, respectively). This study suggests that China's standard for annual PM2.5 (35 μg m−3) in most of the SCB cities might be achieved mainly through controlling SCB emissions (particularly those from industrial and residential activities); however, to meet the WHO guideline and to reduce PM2.5 pollution days and extreme pollution days, both SCB and non-SCB emissions should be greatly reduced. © 2020 Elsevier Ltd
英文关键词Air pollutant transport; Extreme event; PM2.5; Source apportionment
语种英语
scopus关键词Air quality; Housing; Industrial emissions; Weather forecasting; Aerodynamic equivalent diameters; Community multi-scale air qualities; Fine particulate matter; Particulate Matter; PM2.5 concentration; Pm2.5 pollutions; Weather research; World Health Organization; Particles (particulate matter); air quality; concentration (composition); modeling; particulate matter; pollutant source; urban area; urban pollution; air quality; article; China; city; forecasting; particulate matter 2.5; practice guideline; urban area; weather; World Health Organization; China; Sichuan Basin
来源期刊Atmospheric Environment
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/144888
作者单位Institute of New Energy and Low-Carbon Technology, Sichuan University, No. 24, South Section One, First Ring Road, Chengdu, 610065, China; State Key Laboratory of Hydraulics and Mountain River Engineering, Sichuan University, Chengdu, 610065, China; Department of Civil and Environmental Engineering, Louisiana State University, Baton Rouge, LA 70803, United States; Department of Environment, College of Architecture and Environment, Sichuan University, Chengdu, 610065, China; Zachry Department of Civil Engineering, Texas A&M University, College Station, TX 77843, United States; Department of Environmental Science and Engineering, Fudan University, Shanghai, 200438, China
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Qiao X.,Yuan Y.,Tang Y.,et al. Revealing the origin of fine particulate matter in the Sichuan Basin from a source-oriented modeling perspective[J],2021,244.
APA Qiao X..,Yuan Y..,Tang Y..,Ying Q..,Guo H..,...&Zhang H..(2021).Revealing the origin of fine particulate matter in the Sichuan Basin from a source-oriented modeling perspective.Atmospheric Environment,244.
MLA Qiao X.,et al."Revealing the origin of fine particulate matter in the Sichuan Basin from a source-oriented modeling perspective".Atmospheric Environment 244(2021).
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