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DOI10.5194/acp-19-10257-2019
Detection of outflow of formaldehyde and glyoxal from the African continent to the Atlantic Ocean with a MAX-DOAS instrument
Behrens L.K.; Hilboll A.; Richter A.; Peters E.; Alvarado L.M.A.; Hedegaard A.B.K.; Wittrock F.; Burrows J.P.; Vrekoussis M.
发表日期2019
ISSN16807316
起始页码10257
结束页码10278
卷号19期号:15
英文摘要Trace gas maps retrieved from satellite measurements show enhanced levels of the atmospheric volatile organic compounds formaldehyde (HCHO) and glyoxal (CHOCHO) over the Atlantic Ocean. To validate the spatial distribution of this continental outflow, ship-based measurements were taken during the Continental Outflow of Pollutants towards the MArine tRoposphere (COPMAR) project. A Multi-AXis Differential Optical Absorption Spectrometer (MAX-DOAS) was operated aboard the research vessel (RV) Maria S. Merian during cruise MSM58/2. This cruise was conducted in October 2016 from Ponta Delgada (Azores) to Cape Town (South Africa), crossing between Cabo Verde and the African continent. The instrument was continuously scanning the horizon, looking towards the African continent. Enhanced levels of HCHO and CHOCHO were found in the area of expected outflow during this cruise. The observed spatial gradients of HCHO and CHOCHO along the cruise track agree with the spatial distributions from satellite measurements and the Model for OZone and Related chemical Tracers version 4 (MOZART-4) model simulations. The continental outflow from the African continent is observed in an elevated layer, higher than 1000 m, and probably originates from biogenic emissions or biomass burning according to FLEXible PARTicle dispersion model (FLEXPART) emission sensitivities. © 2019 Author(s).
语种英语
scopus关键词atmospheric chemistry; detection method; formaldehyde; outflow; satellite data; spatial distribution; trace gas; volatile organic compound; Africa; Atlantic Ocean; Meria; Vindula arsinoe
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/144760
作者单位Institute of Environmental Physics (IUP-UB), University of Bremen, Bremen, Germany; MARUM-Center for Marine Environmental Sciences, University of Bremen, Bremen, Germany; DLR-Institute of Atmospheric Physics, German Aerospace Center, Oberpfaffenhofen, Germany; Energy Environment and Water Research Center (EEWRC), Cyprus Institute, Nicosia, Cyprus; DLR-Institute for Protection of Maritime Infrastructures, German Aerospace Center, Bremerhaven, Germany
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Behrens L.K.,Hilboll A.,Richter A.,et al. Detection of outflow of formaldehyde and glyoxal from the African continent to the Atlantic Ocean with a MAX-DOAS instrument[J],2019,19(15).
APA Behrens L.K..,Hilboll A..,Richter A..,Peters E..,Alvarado L.M.A..,...&Vrekoussis M..(2019).Detection of outflow of formaldehyde and glyoxal from the African continent to the Atlantic Ocean with a MAX-DOAS instrument.Atmospheric Chemistry and Physics,19(15).
MLA Behrens L.K.,et al."Detection of outflow of formaldehyde and glyoxal from the African continent to the Atlantic Ocean with a MAX-DOAS instrument".Atmospheric Chemistry and Physics 19.15(2019).
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