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DOI10.5194/acp-19-8229-2019
Simulations of black carbon over the Indian region: Improvements and implications of diurnality in emissions
Govardhan G.; Krishnakumari Satheesh S.; Krishna Moorthy K.; Nanjundiah R.
发表日期2019
ISSN16807316
起始页码8229
结束页码8241
卷号19期号:12
英文摘要With a view to improving the performance of WRF-Chem over the Indian region in simulating BC (black carbon) mass concentrations as well as its short-term variations, especially on a diurnal scale, a region-specific diurnal variation scheme has been introduced in the model emissions and the performance of the modified simulations has been evaluated against high-resolution measurements carried out over eight ARFI (Aerosol Radiative Forcing over India) network observatories spread across India for distinct seasons: pre-monsoon (represented by May), post-monsoon (represented by October) and winter (represented by December). In addition to an overall improvement in the simulated concentrations and their temporal variations, we have also found that the effects of prescribing diurnally varying emissions on the simulated near-surface concentrations largely depend on the boundary layer turbulence. The effects are perceived quickly (within about 2-3 h) during the evening-early morning hours when the atmospheric boundary layer is shallow and convective mixing is weak, while they are delayed, taking as much as about 5-6 h, during periods when the boundary layer is deep and convective mixing is strong. This information would also serve as an important input for agencies concerned with urban planning and pollution mitigation. Despite these improvements in the near-surface concentrations, the simulated columnar aerosol optical depth (AOD) still remains largely underestimated vis-à-vis the satellite-retrieved products. These modifications will serve as a guideline for further model-improvement initiatives at a regional scale. © Author(s) 2019.
语种英语
scopus关键词aerosol; black carbon; computer simulation; diurnal variation; emission inventory; numerical model; optical depth; performance assessment; radiative forcing; India
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/144318
作者单位Centre for Atmospheric and Oceanic Sciences, Indian Institute of Science, Bangalore, India; Divecha Centre for Climate Change, Indian Institute of Science, Bangalore, India; Indian Institute of Tropical Meteorology, Pune, India
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Govardhan G.,Krishnakumari Satheesh S.,Krishna Moorthy K.,et al. Simulations of black carbon over the Indian region: Improvements and implications of diurnality in emissions[J],2019,19(12).
APA Govardhan G.,Krishnakumari Satheesh S.,Krishna Moorthy K.,&Nanjundiah R..(2019).Simulations of black carbon over the Indian region: Improvements and implications of diurnality in emissions.Atmospheric Chemistry and Physics,19(12).
MLA Govardhan G.,et al."Simulations of black carbon over the Indian region: Improvements and implications of diurnality in emissions".Atmospheric Chemistry and Physics 19.12(2019).
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