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DOI | 10.5194/acp-19-8931-2019 |
Assessing London CO2; CH4 and CO emissions using aircraft measurements and dispersion modelling | |
Pitt J.R.; Allen G.; Bauguitte S.J.-B.; Gallagher M.W.; Lee J.D.; Drysdale W.; Nelson B.; Manning A.J.; Palmer P.I. | |
发表日期 | 2019 |
ISSN | 16807316 |
起始页码 | 8931 |
结束页码 | 8945 |
卷号 | 19期号:13 |
英文摘要 | We present a new modelling approach for assessing atmospheric emissions from a city, using an aircraft measurement sampling strategy similar to that employed by previous mass balance studies. Unlike conventional mass balance methods, our approach does not assume that city-scale emissions are confined to a well-defined urban area and that peri-urban emissions are negligible. We apply our new approach to a case study conducted in March 2016, investigating CO, For comparison, we also calculate fluxes using a conventional mass balance approach and compare these to the emissions inventory aggregated over the Greater London area. Using this method we derive much higher inventory scale factors for all three gases, as a direct consequence of the failure to account for emissions outside the Greater London boundary. That substantially different conclusions are drawn using the conventional mass balance method demonstrates the danger of using this technique for cities whose emissions cannot be separated from significant surrounding sources. © Author(s) 2019. |
语种 | 英语 |
scopus关键词 | airborne survey; atmospheric plume; carbon dioxide; carbon monoxide; dispersion; emission inventory; flux measurement; Lagrangian analysis; mass balance; methane; England; London [England]; United Kingdom |
来源期刊 | Atmospheric Chemistry and Physics
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/144287 |
作者单位 | School of Earth and Environmental Sciences, University of Manchester, Oxford Road, Manchester, M13 9PL, United Kingdom; Facility for Airborne Atmospheric Measurements (FAAM), Cranfield University, Cranfield, MK43 0AL, United Kingdom; Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, Heslington, York, YO10 5DD, United Kingdom; Met Office, FitzRoy Road, Exeter, EX1 3PB, United Kingdom; School of GeoSciences, University of Edinburgh, Edinburgh, EH9 3FF, United Kingdom |
推荐引用方式 GB/T 7714 | Pitt J.R.,Allen G.,Bauguitte S.J.-B.,et al. Assessing London CO2; CH4 and CO emissions using aircraft measurements and dispersion modelling[J],2019,19(13). |
APA | Pitt J.R..,Allen G..,Bauguitte S.J.-B..,Gallagher M.W..,Lee J.D..,...&Palmer P.I..(2019).Assessing London CO2; CH4 and CO emissions using aircraft measurements and dispersion modelling.Atmospheric Chemistry and Physics,19(13). |
MLA | Pitt J.R.,et al."Assessing London CO2; CH4 and CO emissions using aircraft measurements and dispersion modelling".Atmospheric Chemistry and Physics 19.13(2019). |
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