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DOI10.5194/acp-19-10591-2019
Preliminary results from the FARCE 2015 campaign: Multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of la Réunion
Duflot V.; Tulet P.; Flores O.; Barthe C.; Colomb A.; Deguillaume L.; Vaïtilingom M.; Perring A.; Huffman A.; Hernandez M.T.; Sellegri K.; Robinson E.; O'Connor D.J.; Gomez O.M.; Burnet F.; Bourrianne T.; Strasberg D.; Rocco M.; Bertram A.K.; Chazette P.; Totems J.; Fournel J.; Stamenoff P.; Metzger J.-M.; Chabasset M.; Rousseau C.; Bourrianne E.; Sancelme M.; Delort A.-M.; Wegener R.E.; Chou C.; Elizondo P.
发表日期2019
ISSN16807316
起始页码10591
结束页码10618
卷号19期号:16
英文摘要The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March-April 2015 on the tropical island of La Réunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Réunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio)aerosols and composition of clouds, with a strong focus on the Maïdo mountain slope area. The main observations obtained during this 2-month intensive field campaign are summarized. They include characterizations of forest structure, concentrations of VOCs and precursors emitted by forests, aerosol loading and optical properties in the planetary boundary layer (PBL), formation of new particles by nucleation of gas-phase precursors, ice-nucleating particles concentrations, and biological loading in both cloud-free and cloudy conditions. Simulations and measurements confirm that the Maïdo Observatory lies within the PBL from late morning to late evening and that, when in the PBL, the main primary sources impacting the Maïdo Observatory are of marine origin via the Indian Ocean and of biogenic origin through the dense forest cover. They also show that (i) the marine source prevails less and less while reaching the observatory; (ii) when in the PBL, depending on the localization of a horizontal wind shear, the Maïdo Observatory can be affected by air masses coming directly from the ocean and passing over the Maïdo mountain slope, or coming from inland; (iii) bio-aerosols can be observed in both cloud-free and cloudy conditions at the Maïdo Observatory; (iv) BVOC emissions by the forest covering the Maïdo mountain slope can be transported upslope within clouds and are a potential cause of secondary organic aerosol formation in the aqueous phase at the Maïdo Observatory; and (v) the simulation of dynamics parameters, emitted BVOCs and cloud life cycle in the Meso-NH model are realistic, and more advanced Meso-NH simulations should use an increased horizontal resolution (100m) to better take into account the orography and improve the simulation of the wind shear front zone within which lies the Maïdo Observatory. Using various observations and simulations, this work draws up an inventory of the in situ studies that could be performed in La Réunion and at the Maïdo Observatory. It also aims to develop scientific collaborations and to support future scientific projects in order to better understand the forest-gas-aerosol-cloud system in an insular tropical environment. © 2019 Author(s).
语种英语
scopus关键词aerosol; biogenic emission; boundary layer; cloud; forest cover; nucleation; orography; tropical environment; volatile organic compound; Indian Ocean; Mascarene Islands; Reunion
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/144201
作者单位Laboratoire de l'Atmosphère et des Cyclones (LACy), UMR8105, Université de la Réunion - CNRS, Météo-France, Saint-Denis de La Réunion, France; Observatoire des Sciences de l'Univers de la Réunion (OSUR), UMS3365, Saint-Denis de la Réunion, France; UMR PVBMT, Peuplements Végétaux et Bioagresseurs en Milieu Tropical, Saint-Denis de La Réunion, France; Université Clermont Auvergne, CNRS Laboratoire de Météorologie Physique (LaMP), Clermont-Ferrand, 63000, France; National Oceanic and Atmospheric Administration, Boulder, CO, United States; Cooperative Institute for Research in Environmental Science, Boulder, CO, United States; Department of Chemistry and Biochemistry, University of Denver, Denver, CO, United States; Department of Civil and Environmental Engineering, UC Boulder, Boulder, CO, United States; CNRM, Centre National de la Recherche Météorologique, UMR3589, CNRS - Météo-France, Toulouse, France; Department of Chemistry, University of British Columbia, Vancouver, BC, Canada; Laboratoire des Sciences ...
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Duflot V.,Tulet P.,Flores O.,et al. Preliminary results from the FARCE 2015 campaign: Multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of la Réunion[J],2019,19(16).
APA Duflot V..,Tulet P..,Flores O..,Barthe C..,Colomb A..,...&Elizondo P..(2019).Preliminary results from the FARCE 2015 campaign: Multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of la Réunion.Atmospheric Chemistry and Physics,19(16).
MLA Duflot V.,et al."Preliminary results from the FARCE 2015 campaign: Multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of la Réunion".Atmospheric Chemistry and Physics 19.16(2019).
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