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DOI10.5194/acp-20-11625-2020
Aerosol light absorption and the role of extremely low volatility organic compounds
Tasoglou A.; Louvaris E.; Florou K.; Liangou A.; Karnezi E.; Kaltsonoudis C.; Wang N.; Pandis S.N.
发表日期2020
ISSN16807316
起始页码11625
结束页码11637
卷号20期号:19
英文摘要A month-long set of summertime measurements in a remote area in the Mediterranean is used to quantify aerosol absorption and the role of black and brown carbon. The suite of instruments included a high-resolution aerosol mass spectrometer (HR-ToF-AMS) and a scanning mobility particle sizer (SMPS), both coupled to a thermodenuder and an Aethalometer, a photoacoustic extinctiometer (PAX405), and a single particle soot photometer (SP2). The average refractory black carbon (rBC) concentration during the campaign was 0.14 µg m−3, representing 3 % of the fine aerosol mass. The measured light absorption was two or more times higher than that of fresh black carbon (BC). Mie theory indicated that the absorption enhancement due to the coating of BC cores by nonrefractory material could explain only part of this absorption enhancement. The role of brown carbon (BrC) and other non-BC light-absorbing material was then investigated. A good correlation (R2 = 0.76) between the unexplained absorption and the concentration of extremely low volatility organic compounds (ELVOCs) mass was found. © Author(s) 2020. This work is distributed under the Creative Commons Attribution 4.0 License.
语种英语
scopus关键词absorption; aerosol; black carbon; brown carbon; light; Mediterranean environment; quantitative analysis; summer; volatile organic compound; Mediterranean Region
来源期刊Atmospheric Chemistry and Physics
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/143907
作者单位Department of Chemical Engineering, Carnegie Mellon University, Pittsburgh, PA, United States; Department of Chemical Engineering, University of Patras, Patras, Greece; Institute of Chemical Engineering Sciences (ICE-HT), FORTH, Patras, Greece; Department of Mechanical Engineering, Carnegie Mellon University, Pittsburgh, PA, United States; RJ Lee Group, Inc., Monroeville, PA, United States
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Tasoglou A.,Louvaris E.,Florou K.,et al. Aerosol light absorption and the role of extremely low volatility organic compounds[J],2020,20(19).
APA Tasoglou A..,Louvaris E..,Florou K..,Liangou A..,Karnezi E..,...&Pandis S.N..(2020).Aerosol light absorption and the role of extremely low volatility organic compounds.Atmospheric Chemistry and Physics,20(19).
MLA Tasoglou A.,et al."Aerosol light absorption and the role of extremely low volatility organic compounds".Atmospheric Chemistry and Physics 20.19(2020).
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