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DOI10.1126/science.aba0893
Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells
Ni Z.; Bao C.; Liu Y.; Jiang Q.; Wu W.-Q.; Chen S.; Dai X.; Chen B.; Hartweg B.; Yu Z.; Holman Z.; Huang J.
发表日期2020
ISSN0036-8075
起始页码1352
结束页码1358
卷号367期号:6484
英文摘要We report the profiling of spatial and energetic distributions of trap states in metal halide perovskite single-crystalline and polycrystalline solar cells. The trap densities in single crystals varied by five orders of magnitude, with a lowest value of 2 × 1011 per cubic centimeter and most of the deep traps located at crystal surfaces. The charge trap densities of all depths of the interfaces of the polycrystalline films were one to two orders of magnitude greater than that of the film interior, and the trap density at the film interior was still two to three orders of magnitude greater than that in high-quality single crystals. Suprisingly, after surface passivation, most deep traps were detected near the interface of perovskites and hole transport layers, where a large density of nanocrystals were embedded, limiting the efficiency of solar cells. © 2020 American Association for the Advancement of Science. All rights reserved.
关键词nanocrystalperovskitecrystallinityenergeticshalidemetalperovskitephotovoltaic systemsolar poweranalytic methodArticlechemical compositioncrystal structuredensitydrive level capacitance profilingenergy transfermagnitude estimation methodphysical parameterspriority journalquality controlspatial analysisspectroscopysurface propertythermal admittance spectroscopytrap density of states
语种英语
来源机构Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/133620
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Ni Z.,Bao C.,Liu Y.,et al. Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells[J]. Science,2020,367(6484).
APA Ni Z..,Bao C..,Liu Y..,Jiang Q..,Wu W.-Q..,...&Huang J..(2020).Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells.,367(6484).
MLA Ni Z.,et al."Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells".367.6484(2020).
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