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DOI | 10.1016/j.envpol.2019.01.028 |
Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review | |
Wan, Xin; Kawamura, Kimitaka; Ram, Kirpa; Kang, Shichang; Loewen, Mark; Gao, Shaopeng; Wu, Guangming; Fu, Pingqing; Zhang, Yanlin; Bhattarai, Hemraj; Cong, Zhiyuan | |
发表日期 | 2019 |
ISSN | 0269-7491 |
EISSN | 1873-6424 |
卷号 | 247 |
英文摘要 | Biomass burning (BB) is one of the largest sources of carbonaceous aerosols with adverse impacts on air quality, visibility, health and climate. BB emits a few specific aromatic acids (p-hydroxybenzoic, vanillic, syringic and dehydroabietic acids) which have been widely used as key indicators for source identification of BB-derived carbonaceous aerosols in various environmental matrices. In addition, measurement of p-hydroxybenzoic and vanillic acids in snow and ice cores have revealed the historical records of the fire emissions. Despite their uniqueness and importance as tracers, our current understanding of analytical methods, concentrations, diagnostic ratios and degradation processes are rather limited and scattered in literature. In this review paper, firstly we have summarized the most established methods and protocols for the measurement of these aromatic acids in aerosols and ice cores. Secondly, we have highlighted the geographical variability in the abundances of these acids, their diagnostic ratios and degradation processes in the environments. The review of the existing data indicates that the concentrations of aromatic acids in aerosols vary greatly with locations worldwide, typically more abundant in urban atmosphere where biomass fuels are commonly used for residential heating and/or cooking purposes. In contrast, their concentrations are lowest in the polar regions which are avoid of localized emissions and largely influenced by long-range transport. The diagnostic ratios among aromatic acids can be used as good indicators for the relative amounts and types of biomass (e.g. hardwood, softwood and herbaceous plants) as well as photochemical oxidation processes. Although studies suggest that the degradation processes of the aromatic acids may be controlled by light, pH and hygroscopicity, a more careful investigation, including closed chamber studies, is highly appreciated. (C) 2019 Elsevier Ltd. All rights reserved. |
关键词 | Aromatic acidsBiomass burningTracerAtmospheric aerosolIce core |
学科领域 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS研究方向 | Environmental Sciences |
来源期刊 | ENVIRONMENTAL POLLUTION |
来源机构 | 中国科学院西北生态环境资源研究院 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/112033 |
作者单位 | Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China |
推荐引用方式 GB/T 7714 | Wan, Xin,Kawamura, Kimitaka,Ram, Kirpa,et al. Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review[J]. 中国科学院西北生态环境资源研究院,2019,247. |
APA | Wan, Xin.,Kawamura, Kimitaka.,Ram, Kirpa.,Kang, Shichang.,Loewen, Mark.,...&Cong, Zhiyuan.(2019).Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review.ENVIRONMENTAL POLLUTION,247. |
MLA | Wan, Xin,et al."Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review".ENVIRONMENTAL POLLUTION 247(2019). |
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