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DOI10.1016/j.envpol.2019.01.028
Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review
Wan, Xin; Kawamura, Kimitaka; Ram, Kirpa; Kang, Shichang; Loewen, Mark; Gao, Shaopeng; Wu, Guangming; Fu, Pingqing; Zhang, Yanlin; Bhattarai, Hemraj; Cong, Zhiyuan
发表日期2019
ISSN0269-7491
EISSN1873-6424
卷号247
英文摘要Biomass burning (BB) is one of the largest sources of carbonaceous aerosols with adverse impacts on air quality, visibility, health and climate. BB emits a few specific aromatic acids (p-hydroxybenzoic, vanillic, syringic and dehydroabietic acids) which have been widely used as key indicators for source identification of BB-derived carbonaceous aerosols in various environmental matrices. In addition, measurement of p-hydroxybenzoic and vanillic acids in snow and ice cores have revealed the historical records of the fire emissions. Despite their uniqueness and importance as tracers, our current understanding of analytical methods, concentrations, diagnostic ratios and degradation processes are rather limited and scattered in literature. In this review paper, firstly we have summarized the most established methods and protocols for the measurement of these aromatic acids in aerosols and ice cores. Secondly, we have highlighted the geographical variability in the abundances of these acids, their diagnostic ratios and degradation processes in the environments. The review of the existing data indicates that the concentrations of aromatic acids in aerosols vary greatly with locations worldwide, typically more abundant in urban atmosphere where biomass fuels are commonly used for residential heating and/or cooking purposes. In contrast, their concentrations are lowest in the polar regions which are avoid of localized emissions and largely influenced by long-range transport. The diagnostic ratios among aromatic acids can be used as good indicators for the relative amounts and types of biomass (e.g. hardwood, softwood and herbaceous plants) as well as photochemical oxidation processes. Although studies suggest that the degradation processes of the aromatic acids may be controlled by light, pH and hygroscopicity, a more careful investigation, including closed chamber studies, is highly appreciated. (C) 2019 Elsevier Ltd. All rights reserved.
关键词Aromatic acidsBiomass burningTracerAtmospheric aerosolIce core
学科领域Environmental Sciences & Ecology
语种英语
WOS研究方向Environmental Sciences
来源期刊ENVIRONMENTAL POLLUTION
来源机构中国科学院西北生态环境资源研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/112033
作者单位Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
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GB/T 7714
Wan, Xin,Kawamura, Kimitaka,Ram, Kirpa,et al. Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review[J]. 中国科学院西北生态环境资源研究院,2019,247.
APA Wan, Xin.,Kawamura, Kimitaka.,Ram, Kirpa.,Kang, Shichang.,Loewen, Mark.,...&Cong, Zhiyuan.(2019).Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review.ENVIRONMENTAL POLLUTION,247.
MLA Wan, Xin,et al."Aromatic acids as biomass-burning tracers in atmospheric aerosols and ice cores: A review".ENVIRONMENTAL POLLUTION 247(2019).
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