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DOI | 10.1016/j.scitotenv.2018.03.012 |
Mercury speciation and distribution in a glacierized mountain environment and their relevance to environmental risks in the inland Tibetan Plateau | |
Sun, Xuejun; Zhang, Qianggong; Kang, Shichang; Guo, Junming; Li, Xiaofei; Yu, Zhengliang; Zhang, Guoshuai; Qu, Dongmei; Huang, Jie; Cong, Zhiyuan; Wu, Guangjian | |
发表日期 | 2018 |
ISSN | 0048-9697 |
EISSN | 1879-1026 |
卷号 | 631-632 |
英文摘要 | Glacierized mountain environments can preserve and release mercury (Hg) and play an important role in regional Hg biogeochemical cycling. However, the behavior of Hg in gladerized mountain environments and its environmental risks remain poorly constrained. In this research, glacier meltwater, runoff and wetland water were sampled in Zhadang-Qugaqie basin (ZQB), a typical glacierized mountain environment in the inland Tibetan Plateau, to investigate Hg distribution and its relevance to environmental risks. The total mercury (THg) concentrations ranged from 0.82 to 6.98 ng.L-1, and non-parametric pairwise multiple comparisons of the THg concentrations among the three different water samples showed that the THg concentrations were comparable. The total methylmercury (TMeHg) concentrations ranged from 0.041 to 0.115 ng.L-1, and non-parametric pairwise multiple comparisons of the TMeHg concentrations showed a significant difference. Both the THg and MeHg concentrations of water samples from the ZQB were comparable to those of other remote areas, indicating that Hg concentrations in the ZQB watershed are equivalent to the global background level. Particulate Hg was the predominant form of Hg in all runoff samples, and was significantly correlated with the total suspended particle (TSP) and not correlated with the dissolved organic carbon (DOC) concentration. The distribution of mercury in the wetland water differed from that of the other water samples. THg exhibited a significant correlation with DOC as well as TMeHg, whereas neither THg nor TMeHg was associated with TSP. Based on the above findings and the results from previous work, we propose a conceptual model illustrating the four Hg distribution zones in glacierized environments. We highlight that wetlands may enhance the potential hazards of Hg released from melting glaciers, making them a vital zone for investigating the environmental effect of Hg in glacierized environments and beyond. (C) 2018 Elsevier B.V. All rights reserved. |
关键词 | MercurySpeciationDistributionGlacierized mountain environmentTibetan plateau |
学科领域 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS研究方向 | Environmental Sciences |
来源期刊 | SCIENCE OF THE TOTAL ENVIRONMENT |
来源机构 | 中国科学院西北生态环境资源研究院 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/111952 |
作者单位 | Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China |
推荐引用方式 GB/T 7714 | Sun, Xuejun,Zhang, Qianggong,Kang, Shichang,et al. Mercury speciation and distribution in a glacierized mountain environment and their relevance to environmental risks in the inland Tibetan Plateau[J]. 中国科学院西北生态环境资源研究院,2018,631-632. |
APA | Sun, Xuejun.,Zhang, Qianggong.,Kang, Shichang.,Guo, Junming.,Li, Xiaofei.,...&Wu, Guangjian.(2018).Mercury speciation and distribution in a glacierized mountain environment and their relevance to environmental risks in the inland Tibetan Plateau.SCIENCE OF THE TOTAL ENVIRONMENT,631-632. |
MLA | Sun, Xuejun,et al."Mercury speciation and distribution in a glacierized mountain environment and their relevance to environmental risks in the inland Tibetan Plateau".SCIENCE OF THE TOTAL ENVIRONMENT 631-632(2018). |
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