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DOI10.1016/j.chemosphere.2019.04.047
Anthropogenic and lithogenic fluxes of atmospheric lead deposition over the past 3600 years from a peat bog, Changbai Mountains, China
Guo, Bobo1; Wang, Jing2; Lin, Chunye1; He, Mengchang1; Ouyang, Wei1
发表日期2019
ISSN0045-6535
EISSN1879-1298
卷号227页码:225-236
英文摘要

Ombrotrophic peatlands are widely used to reconstruct atmospheric metal deposition histories. Here, we estimated the long-term atmospheric Pb deposition flux using ombrotrophic peatland data from the Changbai Mountains, northeast China. A peat profile of 320-cm depth was sampled and cut into 164 slices for measurement of Pb and other elements by ICP-MS and ICP-AES and radiometric dating by Pb-210, Cs-137 and C-14. Pb concentration in the peat ranged from 2.18 to 68.33 mg kg(-1), while the atmospheric Pb deposition flux ranged from 0.12 to 12.49 mg m(-2) a(-1). The Little Ice Age (cold and wet climate) led to low Pb concentration, Pb/Sc ratio, and Pb deposition flux (4.40 +/- 0.70 mg kg(-1), 2.04 +/- 0.38, and 0.28 +/- 0.09 mg m(-2) a(-1), respectively). On the other hand, intense volcanic eruptions resulted in high Pb concentration, Pb/Sc ratio, and P flux (54.48 +/- 13.08 mg kg(-1), 7.85 +/- 2.09, and 8.15 +/- 2.85 mg m(-2) a(-1), respectively). In addition, rapid economic development since the 1980s resulted in a gradual increase of anthropogenic Pb concentration from 1.54 mg kg(-1) to 5.85 mg kg(-1); thus, the anthropogenic Pb deposition flux (0.43 +/- 0.21 mg m(-2) a(-1)) was high during this period. In general, peat Pb concentration and atmospheric Pb deposition fluxes in this region have been affected by climate change, volcanic eruptions, and human activities. It was further demonstrated that atmospheric Pb emissions and deposition in China decreased since leaded gasoline was phased out in 2001. The results are critical to understand the geochemistry of Pb and to assess the effects of human activities on atmospheric Pb emissions and deposition in China. (C) 2019 Elsevier Ltd. All rights reserved.


WOS研究方向Environmental Sciences & Ecology
来源期刊CHEMOSPHERE
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/100146
作者单位1.Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China;
2.Wuhan Univ, Sch Resource & Environm Sci, Wuhan 430079, Hubei, Peoples R China
推荐引用方式
GB/T 7714
Guo, Bobo,Wang, Jing,Lin, Chunye,et al. Anthropogenic and lithogenic fluxes of atmospheric lead deposition over the past 3600 years from a peat bog, Changbai Mountains, China[J],2019,227:225-236.
APA Guo, Bobo,Wang, Jing,Lin, Chunye,He, Mengchang,&Ouyang, Wei.(2019).Anthropogenic and lithogenic fluxes of atmospheric lead deposition over the past 3600 years from a peat bog, Changbai Mountains, China.CHEMOSPHERE,227,225-236.
MLA Guo, Bobo,et al."Anthropogenic and lithogenic fluxes of atmospheric lead deposition over the past 3600 years from a peat bog, Changbai Mountains, China".CHEMOSPHERE 227(2019):225-236.
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